Abstract

Searching for new particles beyond the standard model is crucial for understanding several fundamental conundrums in physics and astrophysics. Several hypothetical particles can mediate exotic spin-dependent interactions between ordinary fermions, which enable laboratory searches via the detection of the interactions. Most laboratory searches utilize a macroscopic source and detector, thus allowing the detection of interactions with submillimeter force range and above. It remains a challenge to detect the interactions at shorter force ranges. Here we propose and demonstrate that a near-surface nitrogen-vacancy center in diamond can be utilized as a quantum sensor to detect the monopole–dipole interaction between an electron spin and nucleons. Our result sets a constraint for the electron–nucleon coupling, g_{{mathrm{s}}}^{mathrm{N}}g_{mathrm{p}}^{mathrm{e}}, with the force range 0.1–23 μm. The obtained upper bound of the coupling at 20 μm is g_{{mathrm{s}}}^{mathrm{N}}g_{mathrm{p}}^{mathrm{e}} < 6.24 × 10−15.

Highlights

  • Searching for new particles beyond the standard model is crucial for understanding several fundamental conundrums in physics and astrophysics

  • The experimental investigation of this interaction at force range shorter than 20 μm, remains elusive due to the following challenges: (i) the size of the sensor should be small compared to the micrometer force range; (ii) the geometry of the sensor should allow close proximity between the sensor and the source; (iii) the sensitivity of the sensor should be sufficient for searching or for providing stringent bound for such interaction; (iv) the unwanted noises, such as the magnetic and electric field introduced by environment, should be isolated well

  • 1 λr þ where r is the displacement vector between the electron and nucleon, r 1⁄4 jrj and er = r/r are the displacement and the unit displacement vector, gsN and gpe are the scalar and pseudoscalar coupling constants of the axion-like particles (ALPs) to the nucleon and to the electron, m is mass of the electron, λ = ħ/(mac) is the force range, ma is the mass of the ALP, σ is the Pauli vector of the electron spin, ħ is

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Summary

Introduction

Searching for new particles beyond the standard model is crucial for understanding several fundamental conundrums in physics and astrophysics. A type of hypothetical ultralight scalars, such as axions or axion-like particles (ALPs)[2], has attracted a lot of attention in a wide variety of researches This has been well motivated for decades from the need of cosmology[3], namely, the dark matter candidate[4], the dark energy candidate[5], and from the understanding of the symmetries of charge conjugation and parity in quantum chromodynamics (QCD)[6] as well as predictions from fundamental theories such as string theory[1]. The method can be further extended to investigate other spin-dependent interactions[17] and opens the door for the single-spin quantum sensor to explore new physics beyond the standard model

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