S = 1 antiferromagnetic electron-spin systems on hydrogenated phenalenyl-tessellation molecules for material-based quantum-computation resources

Abstract

A resource state for measurement-based quantum computation is proposed using a material design of S = 1 antiferromagnetic spin chains. Specifying hydrogen adsorption positions on polymerized phenalenyl-tessellation molecules gives rise to formation of graphene zero modes that produce local S = 1 spins or S = 1/2 spins in the required order through exchange interactions. When the S = 1 antiferromagnetic Heisenberg models serve as quantum-computation resources, hydrogen adatoms inducing zero modes can also work as local electron-spin probes in nuclear spin spectroscopy, which could be used for controlling and measuring local spins.