Abstract

The valleys of two-dimensional transition metal dichalcogenides (TMDCs) offer a new degree of freedom for information processing. To take advantage of this valley degree of freedom, on the one hand, it is feasible to control valleys by utilizing different external stimuli, such as optical and electric fields. On the other hand, nanostructures are also used to separate the valleys by near-field coupling. However, for both of the above methods, either the required low-temperature environment or low degree of coherence properties limit their further applications. Here, we demonstrate that all-dielectric photonic crystal (PhC) slabs without in-plane inversion symmetry (C2 symmetry) can separate and route valley exciton emission of a WS2 monolayer at room temperature. Coupling with circularly polarized photonic Bloch modes of such PhC slabs, valley photons emitted by a WS2 monolayer are routed directionally and are efficiently separated in the far field. In addition, far-field emissions are directionally enhanced and have long-distance spatial coherence properties.

Highlights

  • The emergence of two-dimensional transition metal dichalcogenides (TMDCs) has attracted tremendous interest for their possible applications in valleytronics[1,2,3,4,5,6,7,8,9,10,11,12]

  • We demonstrate that two-dimensional alldielectric photonic crystal (PhC) slabs without in-plane inversion symmetry can be used to efficiently separate valley exciton emission of a WS2 monolayer in the far field at room temperature

  • The results demonstrate that by breaking the in-plane inversion symmetry of PhC slabs, circularly polarized states emerge in photonic bands

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Summary

Introduction

The emergence of two-dimensional transition metal dichalcogenides (TMDCs) has attracted tremendous interest for their possible applications in valleytronics[1,2,3,4,5,6,7,8,9,10,11,12]. For this type of PhC slab, paired delocalized Bloch modes with different circular polarizations play a critical role in separating and enhancing directional valley exciton emission and lead to spatial coherence properties of the emission field, which have not been discussed in past studies.

Results
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