Abstract
Time-resolved infrared–ultraviolet (IR–UV) double resonance spectroscopy is employed for rotationally resolved kinetic studies of collision-induced energy transfer between the 4151 and 42 vibrational levels in the ground electronic state of acetylene-d2, C2D2. Second-order rate constants, for intra- and intermolecular V–V transfer and also for V–T,R transfer, are determined.
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