Abstract
We experimentally and theoretically investigate the evolution of the rotational wave packet of N2O at room temperature created by two strong femtosecond laser pulses. The rotational-state populations of the molecule are also calculated after the excitation of the two laser pulses. The results demonstrate that the rotational-state populations and the revival structures can be controlled for the wave packet by precisely adjusting the time delay between the two laser pulses.
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Schedule a callMore From: Journal of Physics B: Atomic, Molecular and Optical Physics
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