Abstract
Time resolved infrared double resonance experiments have been conducted on ozone mixtures in order to determine rotational relaxation rates. A pulsed CO2 laser pumps a ν3 ←ground state transition, while a diode laser is tuned to a hot band transition so that the relaxation process in v3=1 may be observed. Nitrogen, oxygen, rare gas, and self-relaxation rates have been measured, and the temperature dependence of these rates has been investigated over the 200–300 K range.
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