Abstract

Nuclei in the $Z\approx100$ mass region represent the heaviest systems where detailed spectroscopic information is experimentally available. Although microscopic-macroscopic and self-consistent models have achieved great success in describing the data in this mass region, a fully satisfying precise theoretical description is still missing. By using fine-tuned parametrizations of the energy density functionals, the present work aims at an improved description of the single-particle properties and rotational bands in the nobelium region. Such locally optimized parameterizations may have better properties when extrapolating towards the superheavy region. Skyrme-Hartree-Fock-Bogolyubov and Lipkin-Nogami methods were used to calculate the quasiparticle energies and rotational bands of nuclei in the nobelium region. Starting from the most recent Skyrme parametrization, UNEDF1, the spin-orbit coupling constants and pairing strengths have been tuned, so as to achieve a better agreement with the excitation spectra and odd-even mass differences in $^{251}$Cf and $^{249}$Bk. The quasiparticle properties of $^{251}$Cf and $^{249}$Bk were very well reproduced. At the same time, crucial deformed neutron and proton shell gaps open up at $N=152$ and $Z=100$, respectively. Rotational bands in Fm, No, and Rf isotopes, where experimental data are available, were also fairly well described. To help future improvements towards a more precise description, small deficiencies of the approach were carefully identified. In the $Z\approx100$ mass region, larger spin-orbit strengths than those from global adjustments lead to improved agreement with data. Puzzling effects of particle-number restoration on the calculated moment of inertia, at odds with the experimental behaviour, require further scrutiny.

Highlights

  • The stability of superheavy elements (SHE) with atomic numbers Z 104 is entirely due to quantum shell effects

  • The most conspicuous differences between the data and calculations relate to positions of the intruder levels, which are highly dependent on the SO coupling C1∇J of the Skyrme energydensity functionals (EDFs)

  • With the adjusted SO terms, the s.p. energies calculated with UNEDF1SO show the shell gaps that open up at N = 152 and Z = 100

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Summary

Background

Nuclei in the Z ≈ 100 mass region represent the heaviest systems where detailed spectroscopic information is experimentally available. Purpose: By using fine-tuned parametrizations of the energy density functionals, the present work aims at an improved description of the single-particle properties and rotational bands in the nobelium region. Such locally optimized parametrizations may have better properties when extrapolating towards the superheavy region. Methods: Skyrme Hartree-Fock-Bogolyubov and Lipkin-Nogami methods were used to calculate the quasiparticle energies and rotational bands of nuclei in the nobelium region. Starting from the most recent Skyrme parametrization, UNEDF1, the spin-orbit coupling constants and pairing strengths have been tuned, so as to achieve a better agreement with the excitation spectra and odd-even mass differences in 251Cf and 249Bk. Results: The quasiparticle properties of 251Cf and 249Bk were very well reproduced. Puzzling effects of particle-number restoration on the calculated moment of inertia, at odds with the experimental behavior, require further scrutiny

INTRODUCTION
THE MODEL
RESULTS
CONCLUSION
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