Abstract
Rotational assignments are made for the and absorption bands of H2O and D2O, which include the four dipole-allowed components of the lowest 3d Rydberg complex. The absorption spectra are simulated by least-squares optimization of a parameterized rotational Hamiltonian which accounts for rotational-electronic Coriolis effects. The analysis of the spectrum is discussed relative to its context in the Rydberg series.
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