Abstract
Rotational structures and angular momenta of the two observed [2Π3/2]4d gerade Rydberg states of bromine in the region 68 800–72 000 cm−1 have been studied by high resolution resonance enhanced (2+1) multiphoton ionization spectroscopy. The rotational constants have been obtained and the angular momenta of the two [2Π3/2]4d series have been assigned for the first time. These results are further determined and confirmed by computational spectral simulations. The angular momenta of the two observed [2Π3/2]4d Rydberg states are concluded to be Ω=1. Comparison is also made for these two Rydberg states.
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