Abstract

Chiral anomaly, a non-conservation of chiral charge pumped by the topological nontrivial gauge fields, has been predicted to exist in Weyl semimetals. However, until now, the experimental signature of this effect exclusively relies on the observation of negative longitudinal magnetoresistance at low temperatures. Here, we report the field-modulated chiral charge pumping process and valley diffusion in Cd3As2. Apart from the conventional negative magnetoresistance, we observe an unusual nonlocal response with negative field dependence up to room temperature, originating from the diffusion of valley polarization. Furthermore, a large magneto-optic Kerr effect generated by parallel electric and magnetic fields is detected. These new experimental approaches provide a quantitative analysis of the chiral anomaly phenomenon which was inaccessible previously. The ability to manipulate the valley polarization in topological semimetal at room temperature opens up a route towards understanding its fundamental properties and utilizing the chiral fermions.

Highlights

  • Chiral anomaly, a non-conservation of chiral charge pumped by the topological nontrivial gauge fields, has been predicted to exist in Weyl semimetals

  • The condensed matter analogy of Weyl fermions was proposed as the quasiparticle excitations of certain novel gapless topological matter, which is named as Weyl semimetal[4]

  • With time-reversal and inversion symmetries preserved, the Dirac nodes can be formed by two degenerated Weyl nodes, driving the system into a Dirac semimetal, a close sibling of the Weyl semimetal[8]

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Summary

Introduction

A non-conservation of chiral charge pumped by the topological nontrivial gauge fields, has been predicted to exist in Weyl semimetals. With the presence of parallel electric and magnetic fields, Weyl fermions possess a non-conserved chiral charge, that is, the chiral anomaly. In Dirac semimetals, these nodes with opposite chiralities are distinguished by the point-group index or isospin and will split under external magnetic field[9,10,11]. The chiral anomaly raises particular interests owing to its important role in the four-dimensional quantum Hall boundary state[13] It promises intriguing transport phenomena, such as negative magnetoresistance (MR)[14], anomalous Hall effect[15] and nonlocal valley transport[16], holding prospects in valleytronics. The phenomenon of chiral anomaly remains in Dirac semimetals

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