Abstract
All inorganic perovskite CsPbBr3 shows great potential in laser device because of its excellent luminescence characteristics, while the room temperature amplified spontaneous emission (ASE) in a large size CsPbBr3 bulk single crystal is still quite difficult. Herein, we have obtained the room temperature ASE in a sub-centimeter size CsPbBr3 bulk single crystal pumped with the single-photon excitation. Based on the reproducible light path within the CsPbBr3 bulk single crystal, the photonic feedback between the bottom and top facets naturally enhances the population inversion, which exhibits an amplified spontaneous emission threshold of ∼320 µJ/cm2. The blue shift of the ASE peak along with the increased pumping intensity is also observed and ascribed to the reduction of the refractive index and the energy band filling effect. These findings demonstrate the sub-centimeter size CsPbBr3 bulk single crystal to be an excellent candidate as an optical gain media for crystal lasers.
Sign-in/Register to access full text options 
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
