Abstract

We extend the semi-classical trajectory description for the high-order harmonic generation~(HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semi-classical trajectory model with a one-dimensional quantum mechanical simulation, we find that the multi-plateau feature of the HHG spectrum is formed by Umklapp scattering under the electron-hole acceleration dynamics by laser fields. Furthermore, by tracing the scattered trajectories in real-space, the model fairly describes the emitted photon energy and the emission timing of the HHG even in the higher plateau regions. We further consider the loss of trajectories by scattering processes with a mean-free-path approximation and evaluate the HHG cutoff energy as a function of laser wavelength. As a result, we find that the trajectory loss by scattering causes the wavelength independence of the HHG from solids.

Highlights

  • Light-matter interactions have been an important subject in physics from both fundamental and technological points of view [1,2,3,4]

  • We elucidate the role of Umklapp scattering in the high-order harmonic generation (HHG) by comparing the semiclassical trajectory model with the one-dimensional quantum electron dynamics simulation

  • We studied the effect of electron scattering in the HHG from solids based on the semiclassical trajectory description

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Summary

Introduction

Light-matter interactions have been an important subject in physics from both fundamental and technological points of view [1,2,3,4]. A primary example of such phenomena is the high-order harmonic generation (HHG) [11,12,13], which is an extreme photon-upconversion process via strongly nonlinear light-matter interactions. This process has been observed from atomic gases decades ago [14,15], and the gas-phase HHG further opened a novel technology to generate ultrashort laser pulses with attosecond duration, offering a novel avenue to explore ultrafast real-time electron dynamics in matter [16,17,18,19,20,21].

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