Abstract

Perovskite manganites have attracted considerable attention recently due to inhomogeneities in multi-functional properties, observed by various high resolution probes. We present an analysis of the essential role played by complex energy landscapes in the nanometer to micron-scale inhomogeneities observed in perovskite manganites using a model expressed in terms of symmetrized atomic-scale lattice distortion modes. We also discuss the origin for the stability of large metal and insulator domains in the absence of defects. We demonstrate that an intrinsic mechanism, which specifically involves longrange interactions between strain fields, the Peierls-Nabarro energy barrier, and complex energy landscapes with multiple metastable states is responsible for the inhomogeneities in perovskite manganites. This is in contrast to an extrinsic mechanism such as chemical randomness. We highlight experimental results which support our intrinsic, rather than extrinsic, mechanism.

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