Abstract

We present a new design of a robust cavity-enhanced frequency comb-based spectrometer operating under the continuous-filtering Vernier principle. The spectrometer is based on a compact femtosecond Er-doped fiber laser, a medium finesse cavity, a diffraction grating, a custom-made moving aperture, and two photodetectors. The new design removes the requirement for high-bandwidth active stabilization present in the previous implementations of the technique, and allows scan rates up to 100 Hz. We demonstrate the spectrometer performance over a wide spectral range by detecting CO2 around 1575 nm (1.7 THz bandwidth and 6 GHz resolution) and CH4 around 1650 nm (2.7 THz bandwidth and 13 GHz resolution). We achieve absorption sensitivity of 5 × 10-9 cm-1 Hz-1/2 at 1575 nm, and 1 × 10-7 cm-1 Hz-1/2 cm-1 at 1650 nm. We discuss the influence of the scanning speed above the adiabatic limit on the amplitude of the absorption signal.

Highlights

  • Cavity-enhanced laser spectroscopy allows sensitive and selective in-situ detection of molecular species in the gas phase

  • Techniques based on continuous wave (CW) lasers, such as cavity ringdown spectroscopy [1,2], integrated cavity output spectroscopy [3,4], and optical feedback cavity-enhanced absorption spectroscopy [5,6], have already found applications in areas ranging from atmospheric and environmental sensing [7] to breath analysis [8]

  • We present a new, improved approach to continuous-filtering Vernier spectroscopy (CF-VS) based on a compact, free-running Er-doped fiber laser, a fixed diffraction grating, a rotating chopper wheel with a custom-made blade that acts as a moving aperture for selecting the Vernier orders (VOs), and imaging lenses in front of the detectors

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Summary

Introduction

Cavity-enhanced laser spectroscopy allows sensitive and selective in-situ detection of molecular species in the gas phase. Techniques based on continuous wave (CW) lasers, such as cavity ringdown spectroscopy [1,2], integrated cavity output spectroscopy [3,4], and optical feedback cavity-enhanced absorption spectroscopy [5,6], have already found applications in areas ranging from atmospheric and environmental sensing [7] to breath analysis [8]. Their spectral coverage is limited by the CW laser sources. A notable exception is the field-deployed instrument for detection of IO, BrO, NO2 and H2CO in the UV range based on a frequency-doubled femtosecond Ti:Sapphire laser and a low-resolution grating spectrograph [10,11]

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