Road dust trace elements contamination, sources, dispersed composition, and human health risk in Chelyabinsk, Russia

Abstract

There are many sources of urban road dust, such as soil dispersal, emissions of industrial enterprises and thermal power plants, road traffic-related processes. Chelyabinsk was selected as a typical Russian industrial city. This work was the first pollution study of road dust in Chelyabinsk. We examined 125 road dust samples were on the content toxic trace elements (As, Cd, Co, Cr, Cu, Hg, Mn, Ni, Pb, Sb, Sr, and Zn). The concentrations of trace elements in road dust were determined using ICP-MS. Results showed that the metal concentrations in dust were higher than the background value of local soil. The distribution curves of dust were asymmetric, had have two peaks, and showed significant unimodal distribution. The higher share of particles was in the range from 30 … 40 to 250 … 300 μm. The thoracic fraction volume (%) and concentrations of trace elements were higher near metallurgical plants. Cadmium, Сu, Mn, Ni, Sr, Pb and Zn were originated from industry and transport; electrometallurgical plant was source of Cr; Al, Co, and Fe derived from local soils and pavement erosion; As, Hg and Sb were the tracers of coal-fired power stations emission. Ingestion was a major exposure way of toxic elements in the dust. The results suggested that there was no significant potential health risk to both children and adults from exposure to any elements in road dust. The cancer risk for adults and children from exposure to As, Cd, Cr, and Pb was found to be at the acceptable or tolerable level.The study deals with the contamination of potentially toxic trace elements (As, Cd, Co, Cr, Cu, Mn, Ni, Pb, Sb, Sr and Zn) in road dust collected from Chelyabinsk urban area.