Abstract
Study of molar conductivity of several palladium(II) complexes has revealed that cationic acyclic diaminocarbene complexes of palladium(II) containing carbohydrazide fragment in the carbene ligand are capable of reversible cyclization to form a six-membered C,O-chelate. This process is favored by factors enhancing dissociation of the anionic ligand in the starting neutral compound. DFT simulation of cationic carbene complexes of palladium has confirmed possibility of such chelating.
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