Abstract

It is generally believed that anthropogenic aerosols cool the atmosphere; therefore, they offset the global warming resulting from greenhouse gases to some extent. Reduction in sulphate, a primary anthropogenic aerosol, is necessary for mitigating air pollution, which causes atmospheric warming. Here, the changes in the surface air temperature under various anthropogenic emission amounts of sulphur dioxide (SO2), which is a precursor of sulphate aerosol, are simulated under both present and doubled carbon dioxide (CO2) concentrations with a climate model. No previous studies have conducted explicit experiments to estimate the temperature changes due to individual short-lived climate forcers (SLCFs) in different climate states with atmosphere–ocean coupled models. The simulation results clearly show that reducing SO2 emissions at high CO2 concentrations will significantly enhance atmospheric warming in comparison with that under the present CO2 concentration. In the high latitudes of the Northern Hemisphere, the temperature change that will occur when fuel SO2 emissions reach zero under a doubled CO2 concentration will be approximately 1.0 °C, while this value will be approximately 0.5 °C under the present state. This considerable difference can affect the discussion of the 1.5 °C/2 °C target in the Paris Agreement.

Highlights

  • It is generally believed that anthropogenic aerosols cool the atmosphere; they offset the global warming resulting from greenhouse gases to some extent

  • IPCC ­AR51 did not independently estimate radiative forcing by aerosol–cloud interactions caused by anthropogenic sulphate aerosols, the total radiative forcing by sulphate aerosols is clearly a primary component of anthropogenic negative radiative forcing

  • The SSP3-7.0 scenario is published as a Shared Socioeconomic Pathways (SSP)[14,15] future scenario used in the IPCC 6th Assessment Report (AR6) in 2021; the scenario is used as the standard future scenario in the Aerosol Chemistry Model Intercomparison Project (AerChemMIP)[16], which will contribute to IPCC AR6

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Summary

Introduction

It is generally believed that anthropogenic aerosols cool the atmosphere; they offset the global warming resulting from greenhouse gases to some extent. The latest Assessment Report of the Intergovernmental Panel on Climate Change (IPCC AR5)[1] evaluated the instantaneous radiative forcing of anthropogenic sulphate aerosols due to aerosol–radiation interactions to be − 0.40 W m–2, with uncertainty levels of − 0.20 to − 0.60 W m–2 in the global and annual means.

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