Retrospective assessment of indoor radon exposure by measurements of embedded 210Po activity in glass objects

Abstract

In most of the epidemiological studies contemporary radon measurements have been used as surrogates for radon concentrations in past decades even though changes in radon levels and residence may have occurred. Short-lived radon progeny may deposit on available surfaces in dwellings thus giving rise over time to a build up of long-lived progeny. Airborne radon decay products can be deposited and implanted through alpha recoil into the glass surfaces. On glass surface, activities of 210Po may arise as a result of the decay of recoil implanted activity following the alpha decay of surface deposited 218Po or 214Po. Measurement of 210Po implanted on a household glass is a method that can be employed to retrospectively determine the historic level of radon in dwellings. This method is based on the assumption that levels of recoil implanted 210Po in the glass provide a measure of time integrated radon concentration in the environment in which the glass has been located. The surface deposited activity of the radon progenies, which then become implanted in the glass by alpha recoil, is believed to reflect past exposure to airborne activity. Such retrospective measurements on glass are valuable in estimating the human dose derived from radon during the time of exposure. In this paper an account is given of the principles and some field applications of a retrospective technique, using the alpha track detectors, CR-39 and LR-115, to measure 210Po implanted in glass surfaces (surface traps). By using this CR–LR difference technique, the cumulative radon exposure in a dwelling in past decades may be estimated. This method provides reliable radon exposure data as a support to epidemiological studies concerning the health effects of radon exposure in the living environment.