Abstract

In this study, we present results from experiments on the retention of single oil droplets rising through a two-layer density stratification. These experiments confirm the significant slowdown observed in past literature of settling and rising particles and droplets in stratification, and are the first experiments to study single liquid droplets as opposed to solid particles. By tracking the motion of the droplets as they rise through a stratified fluid, we identify two timescales which quantitatively describe this slowdown: an entrainment timescale, and a retention timescale. The entrainment timescale is a measure of the time that a droplet spends below its upper-layer terminal velocity and relates to the length of time over which the droplet's rise is affected by entrained dense fluid. The retention time is a measure of the time that the droplet is delayed from reaching an upper threshold far from the density transition. Both timescales are found to depend on the Froude and Reynolds numbers of the system, Fr $=U_u/(Nd)$ and Re $=\rho_u U_u d/\nu$. We find that both timescales are only significantly large for Fr $\lesssim1$, indicating that trapping dynamics in a relatively sharp stratification arise from a balance between drop inertia and buoyancy. Finally, we present a theoretical formulation for the drag enhancement $\Gamma$, the ratio between the maximum stratification force and the corresponding drag force on the droplet, based on a simple force balance at the point of the velocity minimum. Using our experimental data, we find that our formulation compares well with recent theoretical and computational work by Zhang et al. [J. Fluid Mech. 875, 622-656 (2019)] on the drag enhancement on a solid sphere settling in a stratified fluid, and provides the first experimental data supporting their approach.

Highlights

  • There are many examples of droplets, bubbles, and particles interacting with stratified fluids, including atmospheric and marine pollution [1], oil spills [2,3,4,5,6], oil seeps [7,8], marine snow [9,10,11], and transport and motion of microplastics and marine organisms [12,13,14,15]

  • These two timescales are interconnected by the magnitude of the slowdown (Uu − Umin) relative to the upper-layer terminal velocity (Uu), as well as a constant that reflects the approximately universal form of the recovery of a droplet’s velocity from Umin to Uu. Both timescales are found to depend on the Froude and Reynolds numbers of the system, Froude number (Fr) = Uu/(Nd ) and Re = ρuUud/ν. We find that both timescales are only significantly large for Fr 1, indicating that trapping dynamics in a relatively sharp stratification arise from a balance between drop inertia and buoyancy

  • What is the net effect of stratification on the rising and settling of droplets and particles in a stratified fluid? What are the timescales associated with the induced delay, and how can we parametrize them? And how does a droplet’s motion connect to the physics of the problem? Many prior experimental and numerical studies have been conducted investigating both solid and porous particles settling in stratified fluids, and will be described in detail below

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Summary

Introduction

There are many examples of droplets, bubbles, and particles interacting with stratified fluids, including atmospheric and marine pollution [1], oil spills [2,3,4,5,6], oil seeps [7,8], marine snow [9,10,11], and transport and motion of microplastics and marine organisms [12,13,14,15]. Recent numerical work has suggested the presence of an additional aspect of the stratification-induced force, due to the specific structure of vorticity generated within a stratified fluid [25,26]. What is the net effect of stratification on the rising and settling of droplets and particles in a stratified fluid? Many prior experimental and numerical studies have been conducted investigating both solid and porous particles settling in stratified fluids, and will be described in detail below. The numerical simulations of Bayareh et al [27] showed that the drag coefficient of a settling spherical drop was enhanced in linearly stratified fluids with drop Froude numbers in the range 4 Fr 16 (where Fr is the ratio of the buoyancy timescale to the inertial timescale). A sharp two-layer stratification was studied briefly in their Appendix, for both a rigid particle and a drop, RETENTION OF RISING DROPLETS IN DENSITY

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