Response of a homeotropic nematic liquid crystal to rectilinear oscillatory shear

Abstract

~Received 19 March 1998! The response of a homeotropically aligned nematic liquid crystal layer to oscillatory rectilinear shear ~Couette flow ! was investigated for frequencies f between 0.01 and 200 Hz and layer thickness d between 10 and 130 mm. Below the onset of instability the cell was placed between crossed polars and light transmission was studied using a parallel light beam. The experimental results for the transmitted light intensity agree quantitatively with numerical solutions of the nematodynamic equations for different cell thicknesses, oscillation frequencies, and amplitudes. For frequencies between 25 and 150 Hz the critical oscillation amplitude for the onset of a spatial pattern, observed in polarized white light, could be reached. The pattern consisted of stationary rolls perpendicular to the direction of the oscillation. The experimentally obtained frequency dependence of the critical shear amplitude for the roll instability for different cell thicknesses is compared with an existing theory and the results of numerical calculations. @S1063-651X~98!09411-2# Nematic liquid crystals ~NLCs! exhibit interesting flow phenomena due to the coupling between the local molecular orientation ~director n ˆ! and the velocity field v. The flow properties of NLCs are characterized by Leslie viscosity coefficients a 1 ,...,a6 , two of which a 2(,0) and a 3 are important in describing the coupling between flow and director orientation @1‐4#. In the case of steady, plane, parallel shear flow, e.g., along the x axis with a velocity field v x(z )( v y 5 v z 50) and in the absence of other torques, the director will tend to align in the flow plane ( x-z plane! at a fixed angle u fl 56arctan(a3 /a2) 1/2 with the x axis if a 3,0 ~the 6