Abstract
We apply two different resonant four-wave mixing techniques to transient molecules that are produced by laser vaporization into a supersonic expansion. Degenerate four-wave mixing (DFWM) excitation spectra are obtained for C3 and SiC2 and two-color laser-induced grating spectroscopy (LIGS) is used to produce background-free stimulated-emission-pumping spectra of SiC2.
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