Abstract
Photoelectron energy and angular distributions are measured for the 2+1 multiphoton ionization process H 2 X 1Σ g + (ν = 0, J) + 2hv → E,F 1Σ g +(ν E, J E = J) + hν → H 2 +X 2Σ g + (ν +) + e −, for ν E = 0, 1, or 2 and for J E = 0 or 1 of the inner well of the double-minimum E,F state. Although a strong preference is found for ν + = ν E, the detailed H 2 + vibrational distribution does not exhibit Franck-Condon behavior, and the photoelectron angular distributions vary markedly with both the J E value of the intermediate state and the ν + value of the ion.
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