Abstract

Conditions to get Coherent Anti-Stokes Raman Spectra for strong one-photon-resonance are given. The biharmonic pump was realized by a high power ns-ruby-laser and a broadband dye-laser, focussed together into a small sample cell. Resonance Raman spectra of an extension of some hundreds cm -1 are obtained during one laser shot, thus opening possibilities to investigate excited electronic states or short-living molecules.

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