Abstract

In recent years, freshwater resource contamination by non-point source pollution has become particularly prominent in China. To control non-point source (NPS) pollution, it is important to estimate NPS pollution exports, identify sources of pollution, and analyze the pollution characteristics. As such, in this study, we established the modified export coefficient model based on rainfall and terrain to investigate the pollution sources and characteristics of non-point source total nitrogen (TN) and total phosphorus (TP) throughout the Huangqian Reservoir watershed—which serves as an important potable water source for the main tributary of the lower Yellow River. The results showed that: (1) In 2018, the non-point source total nitrogen (TN) and total phosphorus (TP) loads in the Huangqian Reservoir basin were 707.09 t and 114.42 t, respectively. The contribution ratios to TN export were, from high to low, rural life (33.58%), farmland (32.68%), other land use types (20.08%), and livestock and poultry breeding (13.67%). The contribution ratios to TP export were, from high to low, rural life (61.19%), livestock and poultry breeding (21.65%), farmland (12.79%), and other land use types (4.38%). The non-point source pollution primarily originated from the rural life of the water source protection zone. (2) Non-point source TN and TP pollution loads and load intensities showed significantly different spatial distribution patterns throughout the water source protection area. Specifically, their load intensities and loads were the largest in the second-class protected zone, which is the key source area of non-point source pollution. (3) When considering whether to invest in agricultural land fertilizer control or rural domestic sewage, waste, and livestock manure pollution control, the latter is demonstrably more effective. Thus, in addition to putting low-grade control on agricultural fertilizer loss, to rapidly and effectively improve potable water quality, non-point source pollution should, to a larger extent, also be controlled through measures such as establishing household biogas digesters, introducing village sewage treatment plants, and improving the recovery rate of rural domestic garbage. The research results discussed herein provide a theoretical basis for formulating a reasonable and effective protection plan for the Huangqian Reservoir water source and can potentially be used to do the same for other similar freshwater resources.

Highlights

  • This article is an open access articleRapid population growth and industrial development have created a serious pollution problem that has drastically compromised the safety of potable water sources in China.In particular, eutrophication—which results from excessive nitrogen and phosphorus in the reservoir’s water source—is a significant problem [1,2,3]

  • Given that extensive efforts go toward continuous point source pollution control, potable water sources in China are much more affected by non-point source pollution (NPSP)—which has become a major issue that needs to be urgently addressed [5,6]

  • The results showed that the modified export coefficient model, which was based on regional topography and hydrological conditions, was more representative of actual non-point source pollution

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Summary

Introduction

Rapid population growth and industrial development have created a serious pollution problem that has drastically compromised the safety of potable water sources in China. Eutrophication—which results from excessive nitrogen and phosphorus in the reservoir’s water source—is a significant problem [1,2,3]. Source areas, thereby threatening the health of an extremely large populace [4]. Given that extensive efforts go toward continuous point source pollution control, potable water sources in China are much more affected by non-point source pollution (NPSP)—which has become a major issue that needs to be urgently addressed [5,6]. 60% of China’s lakes have eutrophication problems, and more than 50% of the lakes’ nitrogen and phosphorus originate from non-point source pollution [7,8].

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