Abstract
As the demand for high-performance battery technology increases, the new energy vehicle industry has an urgent need for safer and more efficient battery systems. A model combining five side reactions was developed to be applied to the studies related to this paper. In this paper, the thermal runaway triggering process of Li-ion batteries is simulated, and the relationship between the local heating of the cathode collector surface and the change of the high-temperature area distribution of the diaphragm layer is analyzed. The thermal runaway mechanism is further revealed. Based on the simulation results, the following conclusions can be drawn: phosphonitene compounds can delay the decomposition of the solid electrolyte interphase membrane and reduce the energy yield of battery-side reactions. Compared with the phosphonitene compound, the optimized structure of adding phosphonitene has little effect on the thermal stability of the battery.
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