Research on Temperature Inconsistency of Large-Format Lithium-Ion Batteries Based on the Electrothermal Model

Abstract

Large-format lithium-ion (Li-ion) batteries are increasingly applied in energy storage systems for electric vehicles, owing to their flexible shape design, lighter weight, higher specific energy, and compact layouts. Nevertheless, the large thermal gradient of Li-ion batteries leads to performance degradation and irreversible safety issues. The difference in the highest temperature position at various operational modes makes accurate temperature monitoring complicated. Accordingly, a full understanding of the temperature inconsistency of large-format Li-ion batteries is crucial. In this study, these inconsistent characteristics are analyzed by establishing an electrothermal model and conducting experiments based on an 8-Ah pouch-type ternary Li-ion battery with contraposition tabs. Regarding the characteristic of inhomogeneous temperature distribution, the analysis results demonstrate that it is primarily attributable to the uneven heat generation within the battery system and the effects of the two tabs. For the evolution of the highest temperature position, this study compares the maximum temperature rise of the positive tab and main battery body. The results illustrate that the operating temperature has a greater impact on the maximum temperature rise of the main battery body since its resistance strongly depends on the operating temperature compared to the positive and negative tabs. In addition, the electrothermal model is expected to be employed for the battery thermal management system (BTMS) to mitigate the battery temperature inconsistency.