Abstract

Production of radioisotopes of high specific activity was studied in the JRR-1 reactor using several (n,p) and (n,α) reactions, such as 24Mg(n,p)24Na, 27A1(n,α)24Na, 35Cl(n,p)35S, 35C1(n,α)32P, 58Ni(n,p)58Co, 64Zn (n,p) 64Cu and 67Zn(n,p) 67Cu. The target materials for these reactions were irradiated in several experimental holes of JRR-1 and the radioisotopes formed in the target materials were separated. The amount of the radioisotopes produced and the specific activity were determined, and the possibility of producing high specific activity radioisotopes by these reactions was investigated. The specific activity of the radioisotopes produced by the (n,p) and (n,γ) reactions was more than several hundreds times higher than when produced by the corresponding (n,γ)reactions. Although the yield of the radioisotopes by the former two reactions was fairly small, practical production of high specific activity radioisotopes by this method was thought to be possible, at least for elements of lower atomic number...

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