Abstract

We present an experimental and theoretical study of photoelectron momentum distributions for nitric oxide (NO) and carbon monoxide (CO) molecules generated by intense linearly polarized laser pulses. It is shown that the measured distributions along the outermost backward rescattering caustic are well reproduced by calculations based on the factorization formula with the analytical returning photoelectron wave packet (RWP) recently derived from the adiabatic theory [T. Morishita and O. I. Tolstikhin, Phys. Rev. A 96, 053416 (2017)]. The good agreement between the experimental and theoretical results confirms the validity of the theory for molecular targets. We discuss the dependence of the RWP on the scattering angle not taken into account in previous studies. We also discuss its dependence on the orientation of a molecule with respect to the laser field, which reveals a role of depletion of the initial state for the systems and pulses considered.

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.