Abstract

The Copernicus Atmosphere Monitoring Service (CAMS), operated by the European Centre for Medium-Range Weather Forecasts on behalf of the European Commission, provides daily analyses and 5-day forecasts of atmospheric composition, including forecasts of volcanic sulphur dioxide (SO2) in near-real time. CAMS currently assimilates total column SO2 retrievals from the GOME-2 instruments on MetOp-B and -C and the TROPOMI instrument on Sentinel-5P which give information about the location and strength of volcanic plumes. However, the operational TROPOMI and GOME-2 retrievals do not provide any information about the height of the volcanic plumes and therefore some prior assumptions need to be made in the CAMS data assimilation system about where to place the resulting SO2 increments in the vertical. In the current operational CAMS configuration, the SO2 increments are placed in the mid-troposphere, around 550 hPa or 5 km. While this gives good results for the majority of volcanic emissions, it will clearly be wrong for eruptions that inject SO2 at very different altitudes, in particular exceptional events where part of the SO2 plume reaches the stratosphere. A new algorithm, developed by DLR for GOME-2 and TROPOMI and optimized in the frame of the ESA-funded Sentinel-5P Innovation–SO2 Layer Height Project, the Full-Physics Inverse Learning Machine (FP_ILM) algorithm, retrieves SO2 layer height from TROPOMI in NRT in addition to the SO2 column. CAMS is testing the assimilation of these data, making use of the NRT layer height information to place the SO2 increments at a retrieved altitude. Assimilation tests with the TROPOMI SO2 layer height data for the Raikoke eruption in June 2019 show that the resulting CAMS SO2 plume heights agree better with IASI plume height retrievals than operational CAMS runs without the TROPOMI SO2 layer height information and that making use of the additional layer height information leads to improved SO2 forecasts than when using the operational CAMS configuration. By assimilating the SO2 layer height data the CAMS system can predict the overall location of the Raikoke SO2 plume up to 5 days in advance for about 20 days after the initial eruption.

Highlights

  • Volcanoes can cause serious disruptions for society, not just for people living near them, and further afield when ash and 35 sulphur dioxide (SO2) emitting from highly explosive eruptions reach the upper troposphere or stratosphere, above the clouds, and are transported over vast distances by the prevailing winds

  • The operational Tropospheric Monitoring Instrument (TROPOMI) and Global Ozone Monitoring Experiment-2 (GOME-2) retrievals do not provide any information about the height of the volcanic plumes and some prior assumptions need to be made in the Copernicus Atmosphere Monitoring Service (CAMS) data assimilation system about where to place the resulting SO2 increments in the vertical

  • 100 The SO2 satellite data currently used in the CAMS near-real time (NRT) system are the operational total column-integrated SO2 amount (TCSO2) retrievals from TROPOMI on S5P produced by European Space Agency (ESA) and from the GOME-2 instruments on MetOp-B and MetOp-C produced by Eumetsat's ACSAF

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Summary

10 Abstract

The Copernicus Atmosphere Monitoring Service (CAMS), operated by the European Centre for Medium-Range Weather Forecasts on behalf of the European Commission, provides daily analyses and 5-day forecasts of atmospheric composition, including forecasts of volcanic sulphur dioxide (SO2) in near-real time. The operational TROPOMI and GOME-2 retrievals do not provide any information about the height of the volcanic plumes and some prior assumptions need to be made in the CAMS data assimilation system about where to place the resulting SO2 increments in the vertical. In the current operational CAMS configuration, the SO2 increments are placed in the mid-troposphere, around 550 hPa or 5 km While this gives good results for the majority of volcanic emissions, it will clearly be wrong for eruptions that inject SO2 at 20 very different altitudes, in particular exceptional events where part of the SO2 plume reaches the stratosphere. CAMS is testing the assimilation of these data, making 25 use of the NRT layer height information to place the SO2 increments at a retrieved altitude. By assimilating the SO2 layer height data the CAMS system can predict the overall 30 location of the Raikoke SO2 plume up to 5 days in advance for about 20 days after the initial eruption

Introduction
Datasets
NRT TROPOMI TCSO2 retrieval
FP_ILM NRT TROPOMI Layer Height retrieval
NRT GOME-2 TCSO2 retrieval
IASI SO2 plume altitude retrieval
CAMS model
CAMS data assimilation system
CAMS NRT TCSO2 assimilation configuration (baseline configuration)
Data assimilation configuration for TCSO2 LH data
Sensitivity studies for assimilation of TCSO2 data
Vertical location of the SO2 plume 495
Conclusions
Code and Data availability
680 Acknowledgements
Full Text
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