Abstract
Relaxation oscillation is a nonlinear dynamic phenomenon, commonly observed in viscous-plastic deformation of materials. However, it is the first time that we observed this phenomenon in the viscous flow of borosilicate glass in its super-cooled liquid region. Our investigation identified that the oscillation is caused by the particular microstructure of borosilicate glass. Specifically, the structure of borosilicate glass consists of borate-rich and silicate-rich networks. During the viscous flow, the fast deformation in borate network tends to be localized. However, the network mixing reaction between the borate-rich and silicate-rich networks can slowly relax the fast localized deformation. These two processes occur simultaneously and as a result bring about the relaxation oscillation. Based on this mechanism, the study established a physical constitutive model to predict the relaxation oscillation during the compression of borosilicate glass.
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