Abstract
TheA 2 Π ustate of O2 + was earlier established as an inverted state contrary to previous assumptions. The rotational analysis of a few more bands of theA-X system of O2 + has now been completed. These studies show that the spin-orbit coupling constantA in theA 2 Π ustate gradually varies with the vibrational quantum numberν and is found to be positive forν⩾6. It has also been observed that the spia-rotation interaction is not negligible in theA 2 Π ustate. The spin splitting constantγ is reported for various vibrational levels of this electronic state.
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