Abstract
Conventional <i>N</i>-alkylation methods have been limited to approaches with high energy barriers and low selectivity. In this issue of <i>Chem</i>, MacMillan and co-workers report an innovative halogen abstraction-radical capture (HARC) strategy via metallaphotoredox catalysis that couples strained and hindered alkyl halides with a diverse range of <i>N</i>-nucleophiles.
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