Abstract
Perovskite solar cells (PSCs) have undergone a dramatic increase in laboratory-scale efficiency to more than 25%, which is comparable to Si-based single-junction solar cell efficiency. However, the efficiency of PSCs drops from laboratory-scale to large-scale perovskite solar modules (PSMs) because of the poor quality of perovskite films, and the increased resistance of large-area PSMs obstructs practical PSC applications. An in-depth understanding of the fabricating processes is vital for precisely controlling the quality of large-area perovskite films, and a suitable structural design for PSMs plays an important role in minimizing energy loss. In this review, we discuss several solution-based deposition techniques for large-area perovskite films and the effects of operating conditions on the films. Furthermore, different structural designs for PSMs are presented, including the processing technologies and device architectures.
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