Abstract
Electrophilic nitrogen sources are an increasingly popular class of reagents for the formation of C–N bonds. Recently, a significant number of useful methodologies have been reported, in particular, examples using transition-metal catalysis. This review summarizes the latest developments in this field, with a focus on very recent advances. 1 Introduction 2 Reactions with Stoichiometric Organometallic Reagents 2.1 Organoboron Nucleophiles 2.2 Zirconium Derivatives 2.3 Silicon Derivatives 2.4 Grignard Reagents 2.5 Organozinc Reagents 3 Catalytic Organometallic Species 3.1 C–H Activation Reactions 3.2 Heterocycle Synthesis via Addition/Amination Sequences 3.3 Narasaka–Heck (or Amino-Heck) Reactions 4 Enolates as Nucleophiles 5 Conclusion
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