Abstract
A time evolution of the alignment and structural deformation processes of neutral CS 2 in intense non-resonant nanosecond laser fields (1.9×10 12 W/ cm 2) is derived by ionizing CS 2 using intense circularly polarized femtosecond laser fields (5.5×10 14 W/ cm 2) . From the real-time probing of the momentum distribution of the resultant S 3+ and C 2+ fragment ions produced through the Coulomb explosion induced by the intense femtosecond laser fields, it is identified that the alignment and the structural deformation proceed simultaneously in the nanosecond laser fields.
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