Abstract

The topology of the magnetic interactions of the copper spins in the nitrosonium nitratocuprate $(\text{NO})[\text{Cu}{({\text{NO}}_{3})}_{3}]$ suggests that it could be a realization of the Nersesyan-Tsvelik model [A. A. Nersesyan and A. M. Tsvelik, Phys. Rev. B 67, 024422 (2003)], whose ground state was argued to be either a resonating valence-bond state or a valence-bond crystal. The measurement of thermodynamic and magnetic resonance properties reveals a behavior inherent to low-dimensional spin $S=\frac{1}{2}$ systems and provides indeed no evidence for the formation of long-range magnetic order down to 1.8 K.

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