Abstract
Functionalization of the pentamethylcyclopentadienyl ligands by an electrophilic substitution of hydrogen atoms by [B(C6F5)3] is observed at the Cp* ligands of the alkyne complexes [Cp*2M(η2-PhC2SiMe3], connnected with (M = Ti, formation of 1) or without (M = Zr, formation of 2) loss of the alkyne and molecular hydrogen.
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