Abstract
The reaction of molecular exciplex formation in the gas phase is treated within the framework of the Landau-Zener approximation. The rate constant of exciplex formation is calculated as a function of “system parameter” which depends on the coupling and shape of potential energy surfaces. For a series of model exciplex systems the role of intramolecular vibrations in the formation process and the influence of the coupling strength and the temperature on the formation rate constant is investigated.
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