Abstract
A polymerization reactor system was designed to monitor simultaneously total and individual polymerization rates of liquid and gaseous 1-olefin monomers. Key element of this system is the combination of mass-flow meters and heat flow calorimetry. Polymerization kinetics of propene-and 1-octene-homo-and copolymerizations using the homogeneous methylalumoxane-activated Cp 2ZrCl 2 were investigated. Monomer reactivity ratios and rate constants were determined from calorimetric data.
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