Rayleigh-Brillouin spectra in molecular nitrogen

Abstract

Rayleigh-Brillouin spectra of gaseous ${\mathrm{N}}_{2}$ is measured for light scattered at 15\ifmmode^\circ\else\textdegree\fi{} over a pressure range from 1 to 661 Torr. Spectral profiles are analyzed by means of an appropriate kinetic model. A least-${\ensuremath{\chi}}^{2}$ method determines the optimum values of the theory parameters: total collision frequency and rotational relaxation number. These parameters are compared with values obtained by other methods. Information provided by light-scattering measurements concerning rotational relaxation in dilute systems is discussed.