Abstract
The pressure dependence of the reorientational correlation function for chloroform has been measured by analysis of the Raman 3019 cm − 1 A 1 CH stretching lineshape at 1, 1000, and 2000 bar and 23°C. These reorientational correlation functions were obtained using the method of spectral Fourier deconvolution introduced by Bratos. The results are compared to the correlation times obtained from the NMR deuteron T 1 relaxation times for CDCl 3 and those calculated from high pressure viscosity measurements.
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