Abstract
The Raman spectra of H 2 and D 2 adsorbed on metal–organic framework-5 at various pressures (H 2: 12.8 and 30.3 bar; D 2: 2.2–24.5 bar) and temperatures (H 2: 298 K; D 2: 40–300 K) have been recorded. The shifts observed in the vibrational modes of the gases indicate that physisorption is responsible for the attractive interactions between the gas and the framework; these interactions are larger with respect to those detected for carbon materials.
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