Raman Quantum Beats of Interacting Excitons

Abstract

Quantum beats involving the light hole (lh) and heavy hole (hh) excitons in GaAs are observed using homodyne detection of the transient four-wave mixing response. Unlike the beats of earlier studies, these beats are detected in a geometry for which the effect would be forbidden in the absence of exciton interactions and arise from coherence induced between the lh and hh excitons. The beats demonstrate the existence of the Raman coherence due to interaction, and the decay of the coherence shows the correlation of exciton dephasing rates to be relatively unaffected by the interaction.