Abstract
Raman and infrared spectra of polycrystalline HI and DI in the region of lattice and internal modes for all three phases have been recorded over the temperature range 18 K to the melting point. The temperature dependent Raman and infrared results are consistent with the X-ray and neutron work that two phase transitions occur at HI and DI involving reorientation of the HI and DI molecules as a whole.
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