Radiotoxicity and health risk assessment of 222Rn in groundwater using statistical and Monte Carlo simulation approaches

Abstract

Water is an important natural resource to humans, and itsquality has been a big concern from time immemorial. Water is polluted by the increasing activities of man. Pollutants of major concern include naturally occurring radioactive materials (NORM), heavy and potentially toxic metals, which are ubiquitous in the environment. Naturally occurring radionuclides such as 222Rn are the major precursors of lung and other types of cancer in humans. Exposure to radon in drinking water in excess of 300 pCi/L is treated as a radiological risk, while toxic metals in excess of the World Health Organization (WHO) maximum permissible levels in drinking water are considered both environmental and health risks to humans. A total of 34 groundwater samples were collected in the Akoko area of Ondo State, Nigeria for 222Rn activity concentration determination. The water samples were collected using standard techniques. RAD7 solid-state-detector was utilized for the 222Rn measurements. The results show the activity concentration of 222Rn ranging from 76 pCi/L to 3593 pCi/L with a mean value of 705 ± 76 pCi/L. Inhalation and ingestion doses from 222Rn dissolved in groundwater were evaluated for the infants, children, and adult populations in the study area. Radiological risks were evaluated through statistical and Monte Carlos simulation methods. It can be concluded from this study that there exists a likelihood of radiation-induced health risks due to inhalation of 222Rn from the sampled water.