Abstract
Intense fires occurred in northwestern Spain on 6 September 2000, filling a valley with smoke haze. Aerosol size distribution measurements were performed during 1 day with a thermal inversion, so the aging process of the smoke aerosol could be closely monitored. In 3.5 h, the fine aerosol increased up to 0.06 μm in the geometric median diameter of the fine mode. This aging process enhanced the scattering ability of aerosols. On the basis of several hypotheses on the data obtained, shortwave radiative forcing at surface level, at top level, and in the atmosphere was estimated: instantaneous surface forcing reached up to between −80.4 and −67.4 W/m2, top of the atmosphere (TOA) instantaneous forcing reached up to between −23.4 and +4.9 W/m2, and instantaneous atmosphere forcing reached up to between +44.2 and +85.3 W/m2. The study reveals not only the absorption of solar radiation in the atmosphere by smoke aerosols but also an aerosol‐induced case study, where TOA cooling forcing shifts to warming for specific aerosol single scattering albedo. The daily mean heating rate of the smoke haze was estimated at 5.9 ± 0.6 K/d.
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