Abstract
We demonstrate multiple photon cycling and radiative force deflection on the triatomic free radical strontium monohydroxide (SrOH). Optical cycling is achieved on SrOH in a cryogenic buffer-gas beam by employing the rotationally closed branch of the vibronic transition . A single repumping laser excites the Sr–O stretching vibrational mode, and photon cycling of the molecule deflects the SrOH beam by an angle of via scattering of ∼100 photons per molecule. This approach can be used for direct laser cooling of SrOH and more complex, isoelectronic species.
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More From: Journal of Physics B: Atomic, Molecular and Optical Physics
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