Radiation-induced structure of austenitic steels with different nickel content under neutron irradiation in SM-3 and BOR-60 reactors

Abstract

Comparative studies of the radiation-induced structure of austenitic steels with a nickel content of 10, 20 and 25 wt.%, irradiated sequentially in the SM-3 and BOR-60 reactors, as well as to higher damaging doses in the BOR-60 reactor, have been carried out. The phase composition, dislocation structure, pores, and radiation-induced segregations at grain boundaries were studied by high-resolution analytical methods of transmission electron microscopy, scanning electron microscopy, and atomic probe tomography. The formation of radiation-induced phase precipitates based on nickel has been established, and its volume fraction correlates with the level of radiation-induced segregations, and increases, the higher the nickel content in the steel. The values of barrier strength factors for radiation-induced structural elements in the studied steels are adjusted by calculation and experiment, which makes it possible to determine their contribution to radiation hardening.It is shown that the largest contribution to radiation hardening as a result of neutron irradiation in BOR-60 at high irradiation temperature up to 29 dpa is made by large radiation-induced precipitates of (G + γ') phases. It is shown that with an increase in the damaging dose, the main factor limiting the performance of internal devices will be radiation swelling, since the contribution to the change in properties from radiation-induced phases and radiation defects will not increase due to their density reaching saturation. Steel with 25 wt.% Ni exhibits the lowest level of swelling at high radiation doses, which makes it possible to consider it as a material-candidate for internals for promising VVER reactors with higher temperatures and longer service life.