Abstract
A theoretical expression for the pulsed photoacoustic signal amplitude from NO2–air mixtures is deduced based on a two-level system and the inhomogeneous wave equation, in the limit where the V-T relaxation time is longer than the laser pulse width (low buffer pressure). In this time limit, the photoacoustic signal from NO2, at constant pressure, after excitation by pulses from a Nd:YAG laser at 532 nm, is measured at different buffer pressures. The relaxation rates are obtained by measuring the quenching of visible fluorescence induced by the same laser. The experimental dependence of the photoacoustic signal amplitude on air pressure shows a very good agreement with the model, where the measured relaxation rates are included.
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