Quasifission in Kr84,86 -induced reactions populating superheavy elements

Abstract

Background: Quasifission plays a detrimental role in the synthesis of superheavy elements. Understanding the dynamics of quasifission helps in selecting the optimum target projectile combinations for the synthesis of new superheavy elements.Purpose: The influence of various entrance channel parameters on the quasifission dynamics was explored. Three reactions, $^{84}\mathrm{Kr}+^{198}\mathrm{Pt}$, $^{86}\mathrm{Kr}+^{198}\mathrm{Pt}$, and $^{86}\mathrm{Kr}+^{197}\mathrm{Au}$, expected to be dominated by quasifission, were studied near the Coulomb barrier energies.Methods: The binary fission fragments from the three reactions were detected using the double arm time-of-flight spectrometer CORSET. The mass and total kinetic energy distributions, which are sensitive to the quasifission dynamics, were measured and analyzed for the three reactions.Results: The mass and total kinetic energy distributions of all the three reactions have the characteristics that show the dominance of quasifission. For the reaction $^{84}\mathrm{Kr}+^{198}\mathrm{Pt}$, symmetric quasifission has been found to be relatively more dominant compared to $^{86}\mathrm{Kr}+^{198}\mathrm{Pt}$ reaction. The results have been compared with $^{48}\mathrm{Ca}$- and $^{52}\mathrm{Cr}$-induced reactions, populating nearby nuclei, to understand the evolution of quasifission. An analysis of the timescales in these reactions using a dynamical calculation shows that $^{84}\mathrm{Kr}+^{198}\mathrm{Pt}$ takes a longer time to reach a particular dinuclear shape compared to the other two reactions. The driving potential at the barrier radius also shows a shallower pocket for $^{84}\mathrm{Kr}+^{198}\mathrm{Pt}$ compared to $^{86}\mathrm{Kr}+^{198}\mathrm{Pt}$ and $^{86}\mathrm{Kr}+^{197}\mathrm{Au}$ reactions.Conclusion: The entrance channel isospin difference is found to influence the quasifission dynamics. A higher entrance channel isospin difference may have a larger evolution time, thus driving the systems toward a more symmetric mass split.